Search results for "confined light"

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Coherent Light Harvesting through Strong Coupling to Confined Light

2018

When photoactive molecules interact strongly with confined light modes, new hybrid light–matter states may form: the polaritons. These polaritons are coherent superpositions of excitations of the molecules and of the cavity photon. Recently, polaritons were shown to mediate energy transfer between chromophores at distances beyond the Forster limit. Here we explore the potential of strong coupling for light-harvesting applications by means of atomistic molecular dynamics simulations of mixtures of photoreactive and non-photo-reactive molecules strongly coupled to a single confined light mode. These molecules are spatially separated and present at different concentrations. Our simulations sug…

Physicsconfined lightPhotonLetterta114010405 organic chemistryChromophore010402 general chemistry7. Clean energy01 natural sciences0104 chemical sciencesDelocalized electronMolecular dynamicscoherent light harvestingChemical physicsstrong couplingPolaritonStrong couplingMoleculeGeneral Materials SciencevalokemiaPhysical and Theoretical ChemistryPhysics::Chemical Physicsta116ExcitationJournal of Physical Chemistry Letters
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Coherent Light Harvesting through Strong Coupling to Confined Light

2018

When photoactive molecules interact strongly with confined light modes, new hybrid light-matter states may form: the polaritons. These polaritons are coherent superpositions of excitations of the molecules and of the cavity photon. Recently, polaritons were shown to mediate energy transfer between chromophores at distances beyond the Förster limit. Here we explore the potential of strong coupling for light-harvesting applications by means of atomistic molecular dynamics simulations of mixtures of photoreactive and non-photo-reactive molecules strongly coupled to a single confined light mode. These molecules are spatially separated and present at different concentrations. Our simulations sug…

confined lightcoherent light harvestingstrong couplingvalokemiaPhysics::Chemical Physicspolaritonit
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